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Title:Paramagnetic resonance of the F- and M-centers in alkali halides
Author(s):Holton, William Coffeen
Doctoral Committee Chair(s):Slichter, C. P.
Department / Program:Physics
Discipline:Physics
Degree:Ph.D.
Genre:Dissertation
Subject(s):alkali halides
Abstract:A systematic study by electron spin resonance and electron-nuclear double resonance at low temperatures of the F-center in KCl, NaCl, LiCl, NaF, and LiF is reported, together with an inconclusive observation of the M-center resonance by fast passage resonance techniques. A description of the high sensitivity superheterodyne paramagnetic resonance spectrometer used in the investigation is given. The hyper fine coupling of the F-electron to the nearest eight shells of nuclei surrounding the negative ion vacancy has been measured. A root second moment calculated from the measured hyper fine constants is in agreement with experimental slow passage electron spin resonances 0 The discrepancy between theory and experiment in the case of LiF F-centers is resolved g so that the point-ion lattice model theoretical calculations of Gourary and Adrian are in agreement with the experimental results.
Issue Date:1960
Genre:Dissertation / Thesis
Type:Text
Language:English
URI:http://hdl.handle.net/2142/16626
Other Identifier(s):6247243
Publication Status:published or submitted for publication
Rights Information:© 1960 William Coffeen Holton
Date Available in IDEALS:2010-08-04


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