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Cote, Matthew John 2014-12-15T23:19:21Z 2014-12-15T23:19:21Z 10000-01-01 1988 1988 Time resolved fluorescence depletion (TRFD), a new technique for the study of intramolecular vibrational redistribution, is described. Picosecond time resolution is obtained through the application of picosecond laser pump-probe techniques. A time dependent perturbation theory based description of the interaction of the laser pulses with an ensemble of molecules is presented to show the linear dependence of the signal on the dynamics of the molecular system. Data obtained from the application of this technique to fluorene, butylanine, and 2-amino pyridine in molecular beams are presented as is a description of the apparatus which was used for the experiments. Made available in DSpace on 2014-12-15T23:19:21Z (GMT). No. of bitstreams: 1 8908659.pdf: 5104790 bytes, checksum: 61405fef7022be5b27d13abafae12980 (MD5) Previous issue date: 1988 Embargo set by: Seth Robbins for item 70587 Lift date: Forever Reason: Restricted to the U of I community idenfinitely during batch ingest of legacy ETDs Restricted to the U of I community idenfinitely during batch ingest of legacy ETDs U of I Only 130 p. Thesis (Ph.D.)--University of Illinois at Urbana-Champaign, 1988. http://hdl.handle.net/2142/70421 (UMI)AAI8908659 Chemistry, Physical Picosecond Time-Resolved Studies of IVR: Theory and Applications of Time-Resolved Fluorescence Depletion text Chemistry Chemistry University of Illinois at Urbana-Champaign Dissertation Ph.D.