Femtosecond time and angle-resolved photoelectron spectroscopy of aqueous solutions

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https://hdl.handle.net/2142/55858

Title: Femtosecond time and angle-resolved photoelectron spectroscopy of aqueous solutions
Author(s): Suzuki, Toshinori
Issue Date: 2014-06-17
Keyword(s): Mini-symposium: Spectroscopy in Kinetics and Dynamics
Abstract: We present the femtosecond time- and angle-resolved photoemission spectroscopy of a liquid beam of aqueous solution. A liquid laminar flow 25 micron in diameter is introduced into a high-vacuum photoelectron spectrometer and interrogated using the pump-probe method. The photoelectron kinetic energy distribution is measured by rotating the probe laser polarization with respecto to an electron detection axis with a small detecion solid angle. The observed time- and angle-resolved photoelectron kinetic energies exhibit electron binding energies and characters of transient electronic states of solutes near the liquid surface. The method provides novel information for understanding solution chemistry.
Publisher: International Symposium on Molecular Spectroscopy
Type of Resource: text
Language: en
Permalink: http://hdl.handle.net/2142/55858
DOI: https://doi.org/10.15278/isms.2014.TH01
Copyright and License Information: Copyright 2014 by the authors. Licensed under a Creative Commons Attribution 4.0 International License. http://creativecommons.org/licenses/by/4.0/